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Visualizing Ultrafast Electron Dynamics in Quantum Materials with Tr-ARPES

Hao-Hsiang Jia (郟浩翔)
NSRRC Condensed Matter Physics Group (同步輻射研究中心 凝態物理小組)

Abstract:

We develop time- and angle-resolved photoemission spectroscopy (Tr-ARPES) systems to directly visualize ultrafast electron dynamics by resolving transient electronic states simultaneously in energy, momentum, and time. The operational Tr-ARPES system has already opened a direct window into femtosecond electronic processes in solid-state materials, from excited-state population dynamics and ultrafast electron scattering to photoinduced gap melting. Equipped with an HHG-based EUV probe and OPA pump source, the system provides the broad photon-energy coverage and femtosecond time resolution. Building on this foundation, the TPS 30A Tr-ARPES platform will further expand the reach of ultrafast electron-dynamics studies through enhanced photon flux and circularly polarized femtosecond EUV pulses. These advances allow direct visualization of valley-, orbital-, and symmetry-dependent electronic dynamics in novel quantum materials, offering new insight into nonequilibrium phenomena in condensed matter systems.

Keywords – Tr-ARPES, HHG, ultrafast, dynamics, condensed matter physics

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